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Functionalization of oxabenzonorbornadiene: Manganese(III)-mediated oxidative addition of dimedone

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dc.creator ÇALIŞKAN, Raşit
dc.creator Balci, Metin
dc.creator Sari, Ozlem
dc.date 2017-08-31T21:00:00Z
dc.date.accessioned 2020-10-06T10:49:53Z
dc.date.available 2020-10-06T10:49:53Z
dc.identifier 9a395a6c-1e5f-43f8-af5c-a158b404f73a
dc.identifier 10.1002/poc.3720
dc.identifier https://avesis.sdu.edu.tr/publication/details/9a395a6c-1e5f-43f8-af5c-a158b404f73a/oai
dc.identifier.uri http://acikerisim.sdu.edu.tr/xmlui/handle/123456789/67259
dc.description 3-Chloro-1,2,3,4-tetrahydro-1,4-epoxynaphthalen-2-yl)-3-hydroxy-5,5-dimethylcy-clohex- 2-en-1-one, synthesized by the reaction of oxabenzonorbornadiene with Mn(OAc)(3) and dimedone in the presence of HCl in acetic acid, was submitted to ring-opening reactions with BBr3 and H2SO4. Reaction with BBr3 yielded 2 products, a 5-membered ring and an 8-membered ring, with the former being the major product. However, the H2SO4-supported reaction exclusively formed an 8-membered ring. The mechanism of formation of these products was supported by theoretical calculations.
dc.language eng
dc.rights info:eu-repo/semantics/openAccess
dc.title Functionalization of oxabenzonorbornadiene: Manganese(III)-mediated oxidative addition of dimedone
dc.type info:eu-repo/semantics/article


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