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Can sulfur-containing molecules solvate/ionize HCl? Solid state solvation of HCl on/in methanethiol clusters/nanoparticles

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dc.creator Balci, F. Mine
dc.creator Uras-Aytemiz, Nevin
dc.creator Devlin, J. Paul
dc.date 2019-11-21T00:00:00Z
dc.date.accessioned 2021-12-03T11:21:01Z
dc.date.available 2021-12-03T11:21:01Z
dc.identifier 47296217-d6a1-45e4-98f2-c39dfc6505b5
dc.identifier 10.1063/1.5126029
dc.identifier https://avesis.sdu.edu.tr/publication/details/47296217-d6a1-45e4-98f2-c39dfc6505b5/oai
dc.identifier.uri http://acikerisim.sdu.edu.tr/xmlui/handle/123456789/91253
dc.description Solvation of HCl at <100 K at the surface of nanoparticles of methanethiol, a sulfur derivative of methanol, was investigated by FTIR spectroscopy and on-the-fly molecular dynamics as implemented in the density functional code QUICKSTEP (which is part of the CP2K package). Some of the results have been further checked with MP2-level ab initio calculations. Unlike the HCl-CH3OH system that has been examined before, HCl on the surface or within methanethiol nanoparticles does not achieve an ionized form. Requirements for acid solvation/ionization are discussed in context with the results for methanol clusters. Published under license by AIP Publishing.
dc.language eng
dc.rights info:eu-repo/semantics/closedAccess
dc.title Can sulfur-containing molecules solvate/ionize HCl? Solid state solvation of HCl on/in methanethiol clusters/nanoparticles
dc.type info:eu-repo/semantics/article


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